Optically stimulated luminescence (OSL) is a known property in many scintillators, and investigating the branching ratio of thermalized carriers to this photon-emission mechanism could aid both scintillator development and OSL-based dosimetry. We present a novel method for determining the branching ratio of thermalized carriers to OSL in scintillators while monitoring the energy deposition from 511 keV gamma photons on an event-by-event basis. We demonstrate the method using a cerium-doped lutetium oxyorthosilicate (LYSO:Ce) crystal, and validate that the observed signal indeed originates from OSL photons by estimating the lifetime of the OSL traps, which is consistent with values found in the literature. We report a branching ratio of thermalized carriers to the OSL traps in LYSO:Ce of (1.0±0.2)% upon excitation with 511 keV gamma photons, using a one-trap-one-recombination-center model.
Jensen, M., Martinez Turtos, R., Julsgaard, B., Schulz, V., Balling, P., Gundacker, S. (2022). A novel method for investigating optically stimulated luminescence in scintillators. JOURNAL OF LUMINESCENCE, 251 [10.1016/j.jlumin.2022.119237].
A novel method for investigating optically stimulated luminescence in scintillators
Martinez Turtos R.;Gundacker S.
2022
Abstract
Optically stimulated luminescence (OSL) is a known property in many scintillators, and investigating the branching ratio of thermalized carriers to this photon-emission mechanism could aid both scintillator development and OSL-based dosimetry. We present a novel method for determining the branching ratio of thermalized carriers to OSL in scintillators while monitoring the energy deposition from 511 keV gamma photons on an event-by-event basis. We demonstrate the method using a cerium-doped lutetium oxyorthosilicate (LYSO:Ce) crystal, and validate that the observed signal indeed originates from OSL photons by estimating the lifetime of the OSL traps, which is consistent with values found in the literature. We report a branching ratio of thermalized carriers to the OSL traps in LYSO:Ce of (1.0±0.2)% upon excitation with 511 keV gamma photons, using a one-trap-one-recombination-center model.
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